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Singular Stability Estimates for Passive Gamma Emission Tomography of Spent Nuclear Fuel

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Abstract

We study the joint recovery of attenuation and source coefficients from the attenuated X-ray transform, motivated by passive gamma emission tomography of spent nuclear fuel. Both coefficients are constant on known, disjoint disks of equal radius representing fuel rods. The surrounding moderator has known attenuation and zero source. We use tangential singularities of the data to give a sufficient condition on the geometry and coefficients for unique joint reconstruction from full data. For rods arranged on parallel rows separated by more than one rod diameter, with source coefficients uniformly bounded away from zero, we derive explicit reconstruction formulas and stability estimates for both coefficients. The estimates use a singular seminorm determined by two functionals per rod, computed from angular data near selected tangencies. Numerical experiments examine the approximation of these functionals from discretized data.

Introduction

Passive gamma emission tomography (PGET) is a non-invasive technique for verifying the internal configuration of spent nuclear fuel assemblies [2]. Gamma rays emitted by the fuel rods are attenuated as they pass through the rods and the moderator before reaching a row of collimated gamma-ray detectors. Mathematically, these measurements are modeled by the attenuated X-ray transform (AtRT) Raf\mathcal{R}_a f, where ff describes the emission and aa the attenuation in a domain Ω\Omega.

In standard emission tomography, the attenuation is often treated as known, at least approximately, and only the source is recovered. Reconstruction methods include iterative approaches [25, 10] and, for the attenuated X-ray transform, Novikov’s inversion formula [19]. In PGET, both aa and ff are unknown and both are of interest. Their joint recovery from the AtRT is also known as the SPECT identification problem [3] and has been studied since the late 1970s [5, 15]. The problem is not uniquely solvable in general, so unique recovery requires additional structure.

We impose geometric and material assumptions motivated by the design of nuclear fuel assemblies. The domain is a fixed disk containing finitely many disjoint smaller disks of equal radius at known locations. The smaller disks represent cross-sections of fuel rods. We model aa and ff as constant on each rod, with known attenuation and zero source in the moderator. Holman and Richardson [12] analyzed the singularities associated with tangential rays and recovered attenuation jumps under a non-cancellation condition.

Our contribution has two parts. First, we give a condition involving a common tangent and a second emitting rod that ensures non-cancellation on an open family of tangencies of a rod with a nonzero attenuation jump (Lemma 3.3). This gives a sufficient condition for recovery from full data (Theorem 3.5). Second, for rods on sufficiently separated parallel rows with strictly positive rod sources, we select tangencies at which non-cancellation holds uniformly over the parameter space. These tangencies give explicit reconstruction formulas and stability estimates for both coefficients in a specific singular data seminorm (Theorem 4.7). The analysis does not include noise or scattering. Stability remains open when the assembly contains a non-emitting rod, such as fresh nuclear fuel or a special absorber rod.

Related literature

When a=0a = 0, the AtRT is the classical Radon transform. For known constant attenuation in a known convex domain, removing the factor determined by the ray’s exit point gives the exponential Radon transform [16], for which explicit inversion formulas are available [26]. Hertle [9] studied the identification of an unknown constant attenuation parameter when the source is also unknown. Solmon [23] studied the corresponding identification problem, including the role of radial symmetry. Novikov established an explicit inversion formula [19] and a range characterization [18] for the two-dimensional attenuated X-ray transform. Natterer [17] derived a closely related exact inversion formula using a different approach. Boman and Strömberg [4] gave an alternative proof of Novikov’s inversion formula and extended it to a broader class of weighted Radon transforms. Kunyansky [14] developed a noniterative SPECT reconstruction algorithm based on Novikov’s inversion formula for known, spatially varying attenuation. An earlier approach used the theory of AA-analytic functions [ABK98]. Surveys include [8, 20 Zho24, 21].

Dicken [6] studied joint recovery using the stability and mapping properties of the AtRT in LpL^p and Sobolev spaces, together with nonlinear Tikhonov regularization. Stefanov [24] studied uniqueness, stability, and the linearized problem, and also demonstrated non-uniqueness when both coefficients are radial. Holman and Richardson [11] established unique recovery under a piecewise constant assumption on the attenuation and with a sufficiently regular source. Their subsequent work [12] treated piecewise smooth sources and real-analytic interfaces under a non-cancellation condition.

PGET has been developed for nuclear safeguards and the verification of spent nuclear fuel [30, 28], and has been approved by the International Atomic Energy Agency (IAEA) since 2017 [30]. A reconstruction method used in practice combines an iterative Levenberg–Marquardt trust-region algorithm with physical constraints and variational regularization [2, 27, 28]. Other methods have been developed, for example in [SHG15, WMD+17, FADL+21]. The fixed rod geometry of PGET motivates our analysis of uniqueness and stability.

Organization of the article

This article addresses two questions in the PGET disk model.

  1. When can non-cancellation be established from the geometry and the coefficient assumptions?

  1. How stable are the recovered attenuation and source with respect to perturbations of the data?

§ 3 addresses the first question, and § 4 addresses the second. We present related numerical experiments in § 5 to help illustrate some of the presented concepts and theoretical results. These codes are also available in https://github.com/tommheik/PGET_stability.

The following diagram summarizes the structure of the proofs of the two main results.

Lemma 2.12 \hspace{4em} [19]

Lemma 2.8 \hspace{2em} → Corollary 2.14 → Lemma 3.3 → Theorem 3.5 \hspace{2em} Lemma 2.3

Remark 2.9 \hspace{2em} Proposition 2.19 ← Lemma 2.5

Corollary 2.14 → Proposition 4.4 → Theorem 4.7 ← Remark 2.18

Lemma 2.7

We prove Theorem 3.5 in § 3. The main step is Lemma 3.3, which combines the chord formulas of Lemma 2.8 with the tangential trace representation in Corollary 2.14 to show that the non-cancellation coefficient does not vanish identically along a family of simple tangencies near a common tangent. The singular identities of Proposition 2.19, based on [12], then determine the attenuation. Once the attenuation is known, Novikov’s inversion formula [19] recovers the source.

The proof of Theorem 4.7 in § 4 uses the admissible tangencies constructed in Proposition 4.4. Under the row-separation assumption, this proposition provides, for every rod, a tangency at which the tangential trace vanishes. The positive lower bound on the rod sources therefore gives a uniform non-cancellation bound. Combining the identities of Proposition 2.19 with the geometric bounds of Lemma 2.7 and the seminorm estimates of Remark 2.18 yields the stability estimates.

Measurement geometry and mathematical model

We introduce the forward model and the fixed geometry, then describe tangencies and backward-ray chords used in reconstruction. We also specify the coefficient space and the singular data functionals.

The attenuated X-ray transform

We work in the planar cross-section R2\mathbb{R}^{2}. For an angle ω∈[0,2π)\omega\in[0,2\pi), we set

θ(ω)=(cos⁡ωsin⁡ω)∈S1,θ⊥(ω)=∂ωθ(ω)=(−sin⁡ωcos⁡ω).\theta(\omega)=\begin{pmatrix}\cos\omega\\ \sin\omega\end{pmatrix}\in S^{1}, \qquad\theta^{\perp}(\omega)=\partial_{\omega}\theta(\omega)=\begin{pmatrix}-\sin\omega\\ \cos\omega\end{pmatrix}.

Angles are understood modulo 2π2\pi. Thus, the space of angle pairs is the torus (R/2πZ)2(\mathbb{R}/2\pi\mathbb{Z})^{2}, represented by [0,2π)2[0,2\pi)^{2}. Angular neighborhoods and one-sided limits are expressed using local real representatives. The directed line through x∈R2x \in\mathbb{R}^{2} with direction θ(ω)\theta(\omega) is

L(x,θ(ω)):={x+tθ(ω):t∈R}.L(x,\theta(\omega)):=\{x+t\theta(\omega):t\in\mathbb{R}\}.

The attenuation aa and source ff are bounded nonnegative measurable functions that vanish outside the bounded domain Ω\Omega specified below. The beam transform of aa is

Da(x,θ(ω))=∫0∞a(x+ρθ(ω)) dρ.(1)Da(x,\theta(\omega))=\int_{0}^{\infty}a(x+\rho\theta(\omega))\,d\rho. \tag*{(1)}

The beam transform measures the attenuation accumulated along the forward ray from xx in the direction θ(ω)\theta(\omega). The attenuated X-ray transform (AtRT) of ff with attenuation aa is

Raf(x,θ(ω))=∫−∞∞f(x+tθ(ω))e−Da(x+tθ(ω),θ(ω)) dt.R_a f(x,\theta(\omega))=\int_{-\infty}^{\infty}f(x+t\theta(\omega))e^{-D_a(x+t\theta(\omega),\theta(\omega))}\,dt.

A change of variable shows that

Raf(x+sθ,θ)=Raf(x,θ),s∈R.R_a f(x+s\theta,\theta)=R_a f(x,\theta),\qquad s\in\mathbb{R}.

Thus, the data depend only on the oriented line, independently of the point chosen to represent it.

For a bounded convex Lipschitz domain Ω⊂R2\Omega\subset\mathbb{R}^2 with unit outward normal ν\nu, let

Γ−={(x,θ)∈∂Ω×S1:θ⋅ν(x)≤0}.\Gamma^-=\{(x,\theta)\in\partial\Omega\times\mathbb{S}^1:\theta\cdot\nu(x)\leq0\}.

The transport equation

θ⋅∇xu(x,θ)+a(x)u(x,θ)=f(x),(x,θ)∈Ω×S1,u∣Γ−=0,(2)\theta\cdot\nabla_xu(x,\theta)+a(x)u(x,\theta)=f(x),\qquad(x,\theta)\in\Omega\times\mathbb{S}^1,\qquad u|_{\Gamma^-}=0, \tag*{(2)}

has a solution uu given by

u(x,θ(ω))=∫−∞0f(x+tθ(ω))exp⁡(−∫t0a(x+(t−ρ)θ(ω)) dρ) dt.(3)u(x,\theta(\omega))=\int_{-\infty}^{0}f(x+t\theta(\omega))\exp\left(-\int_t^0a(x+(t-\rho)\theta(\omega))\,d\rho\right)\,dt. \tag*{(3)}

see [12 Section 2]. For every x∈R2x\in\mathbb{R}^2 and ω∈[0,2π)\omega\in[0,2\pi), a change of variables in (3) gives the backward-ray representation

u(x,θ(ω))=∫0∞f(x−sθ(ω))exp⁡(−∫0sa(x−σθ(ω)) dσ) ds.(4)u(x,\theta(\omega))=\int_0^\infty f(x-s\theta(\omega))\exp\left(-\int_0^s a(x-\sigma\theta(\omega))\,d\sigma\right)\,ds. \tag*{(4)}

For y∈R2y\in\mathbb{R}^2, θ∈S1\theta\in\mathbb{S}^1, and s≥0s\geq0, the beam transform satisfies

Da(y−sθ,θ)=∫0sa(y−σθ) dσ+Da(y,θ).D_a(y-s\theta,\theta)=\int_0^s a(y-\sigma\theta)\,d\sigma+D_a(y,\theta).

Consequently, setting s=−ts=-t and using (4) give

∫−∞0f(y+tθ)e−Da(y+tθ,θ) dt=e−Da(y,θ)∫0∞f(y−sθ)exp⁡(−∫0sa(y−σθ) dσ) ds=e−Da(y,θ)u(y,θ).\begin{aligned} \int_{-\infty}^{0}f(y+t\theta)e^{-D_a(y+t\theta,\theta)}\,dt=e^{-D_a(y,\theta)}\int_0^\infty f(y-s\theta)\exp\left(-\int_0^s a(y-\sigma\theta)\,d\sigma\right)\,ds \\ &=e^{-D_a(y,\theta)}u(y,\theta). \end{aligned}

Splitting the integral defining RafR_af at t=0t=0 yields

Raf(y,θ)=e−Da(y,θ)u(y,θ)+∫0∞f(y+tθ)e−Da(y+tθ,θ) dt.R_af(y,\theta)=e^{-D_a(y,\theta)}u(y,\theta)+\int_0^\infty f(y+t\theta)e^{-D_a(y+t\theta,\theta)}\,dt.

Let x∈∂Ωx\in\partial\Omega be a point where the outward normal ν(x)\nu(x) is defined, and suppose that θ⋅ν(x)≥0\theta\cdot\nu(x)\geq0. By convexity, the forward ray {x+tθ:t>0}\{x+t\theta:t>0\} does not enter Ω\Omega. The zero extension of aa gives Da(x,θ)=0D_a(x,\theta)=0. The forward source integral also vanishes. The data and the solution uu therefore satisfy

Raf(x,θ)=u(x,θ).R_af(x,\theta)=u(x,\theta).

Geometric setting of PGET

Fuel rods are enclosed in metal cladding and arranged in assemblies containing dozens or hundreds of rods. Assembly designs include rectangular and hexagonal arrangements, water channels of different sizes, and partial-length rods. For details, see [28]. For a specified assembly and axial slice, the rod positions and diameters are known. Gamma-ray measurements are acquired with collimated detectors located on a ring outside the assembly. Figure 1 shows a PGET device.

PGET device with its outer cover removed and a shortened dummy assembly

Figure 1. PGET device with its outer cover removed and a shortened dummy assembly. Measurements are collected around a horizontal slice of the assembly. Photograph by Dean Calma / IAEA.

We model the slice as disks of equal radius with constant coefficients, surrounded by a moderator with known attenuation and zero source. The model omits cladding, axial variation, scattering, and the finite collimator response. Known moderator-filled positions, including water channels and partial rods fully outside the field of view, belong to the moderator. Every other non-emitting rod remains a rod in the coefficient model. We also assume that the location of the assembly within the domain is known.

We now specify this geometry. Fix an outer radius rout>0r_{\mathrm{out}} > 0 and let Ω=B(0,rout)\Omega= B(0,r_{\mathrm{out}}), with boundary

∂Ω={x(ψ):x(ψ)=rout(cos⁡ψ,sin⁡ψ), ψ∈[0,2π)}.\partial\Omega= \{x(\psi) : x(\psi) = r_{\mathrm{out}}(\cos\psi,\sin\psi),\ \psi\in[0,2\pi)\}.

Fix the number of rods K≥2K \ge2, their radius r>0r > 0 and centers c1,…,cKc_1,\ldots,c_K such that the closed disks

B‾q=B(cq,r)⊂Ω,q=1,…,K,\overline{B}_q = B(c_q,r) \subset\Omega,\qquad q=1,\ldots,K,

are pairwise disjoint. Equivalently, ∣cq−cq′∣>2r|c_q-c_{q'}| > 2r for q≠q′q \ne q' and ∣cq∣+r<rout|c_q|+r < r_{\mathrm{out}} for every qq. The rod boundaries are ∂Bq\partial B_q, q=1,…,Kq=1,\ldots,K, and we write Ω0=Ω∖⋃q=1KB‾q\Omega_0 = \Omega\setminus\bigcup_{q=1}^{K}\overline{B}_q for the moderator region. The disks B1,…,BKB_1,\ldots,B_K model the fuel or metal rods, and Ω0\Omega_0 models the surrounding water. We illustrate this in Figure 2. These parameters define the geometry

Measurement geometry with disjoint rods in the moderator

Figure 2. Measurement geometry with disjoint rods BqB_q in the moderator Ω0\Omega_0. The angle ψ\psi specifies x(ψ)x(\psi), and ω\omega specifies the direction of L(ψ,ω)L(\psi,\omega).

G=(rout,r,{cq}q=1K),(5)\mathcal{G} = \left(r_{\mathrm{out}},r,\{c_q\}_{q=1}^{K}\right), \tag*{(5)}

which remains fixed throughout the article. For (ψ,ω)∈[0,2π)2(\psi,\omega) \in[0,2\pi)^2, we abbreviate L(ψ,ω):=L(x(ψ),θ(ω))L(\psi,\omega) := L(x(\psi),\theta(\omega)).

Tangencies of the rods

We regard the angular parameter space as the torus (R/2πZ)2(\mathbb{R}/2\pi\mathbb{Z})^2 and use [0,2π)2[0,2\pi)^2 for representatives of its points.

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