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Bichromatic light-induced electronic torques on the Néel vector in Rashba magnetic multipoles from pp-wave magnets to ii-wave altermagnets

Abstract

Light can control magnetic order on ultrafast timescales, but for a two-dimensional magnet with an out-of-plane order parameter N∥z^\boldsymbol N\parallel\hat z, the inverse Faraday field is collinear with N\boldsymbol N and gives no transverse torque. Here we show that bichromatic (ω,bω)(ω,bω) light generates electronic torques perpendicular to N\boldsymbol N in Rashba-coupled magnetic multipoles, from pp-wave (n=1n=1) magnets to ii-wave (n=6n=6) altermagnets. Beyond high-frequency effective fields, we evaluate the exact Floquet response and the generalized torque per occupied electron, for prescribed occupations. The momentum-dependent exchange terms dominate this Fermi-sea torque and remove the leading-order zeros (amplitude-ratio blindspots) of the momentum-independent field in the channels tested. For out-of-plane N\boldsymbol N, rotational symmetry permits a transverse torque only if gcd⁡(n,b+1)=1\gcd(n,b+1)=1 for counter-rotating beams or gcd⁡(n,b−1)=1\gcd(n,b-1)=1 for co-rotating beams. For in-plane N\boldsymbol N, the Fermi sea also gives a torque component along z^\hat z that the momentum-independent field cannot produce. We classify the active channels, with n=1,…,6n=1,\dots,6 and b=1,…,7b=1,\dots,7, by frequency scaling and origin (cycle-averaged versus oscillating exchange). As a control, a Rashba ferromagnet (n=0n=0) has one symmetry-allowed out-of-plane channel and a weak in-plane response without a selection rule. Finite-momentum occupied-state physics is therefore essential for light-driven torques in unconventional magnets, and the exact Floquet calculation validates and extends the high-frequency description.

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