WorksPhysics and Astronomy
Stripe antiferromagnetic order and spin dynamics in the Shastry-Sutherland Ising compound Er2Be2GeO7
Abstract · v1
In rare-earth compounds, the interplay between geometric frustration and unusual single-ion anisotropy caused by the crystal electric field often leads to exotic magnetic phases. Here, we investigate the magnetic properties of the rare-earth Shastry-Sutherland compound ErBeGeO using bulk measurements and neutron scattering down to sub-Kelvin temperatures. A stripe-like antiferromagnetic order with locally tilted Er moments is revealed by time-of-flight neutron powder diffraction, accompanied with a -shape specific-heat anomaly at K. The temperature dependence of the magnetic peak intensity corresponding to the ordered moment of Er approximates to the two-dimensional Ising universality class. Thermal- and cold-neutron inelastic scattering experiments demonstrate that the strong Ising anisotropy originates from the local crystal electric field, and reveal gapped magnetic excitations with weak dispersion in the ordered state. Mean-field random-phase approximation with inequivalent nearest-neighbor couplings accounts well for the collective excitations, while classical Monte Carlo simulations yield the fractional and magnetization plateaus. Our work provides a comprehensive description of the spin correlations in ErBeGeO with a particular focus on the classical origin of its fractional magnetization plateaus.
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