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A density-uniform condensate bound for dilute Bose gases

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Abstract

For each fixed bounded measurable, nonnegative, radial interaction of finite range in three dimensions that is not zero almost everywhere, we prove a positive lower bound on the constant-orbital condensate fraction that is uniform over all sufficiently small densities and all temperatures between zero and the square of the density. The interaction and density remain fixed in the thermodynamic limit.

The model and the uniform bound

For a homogeneous gas, Bose–Einstein condensation means that one orbital contains a positive fraction of all particles in the equilibrium state. We consider the spatially constant orbital and keep both the physical interaction and a positive density fixed as the volume grows. The bound below uses the same positive fraction throughout a sufficiently dilute interval of densities.

Let v:R3→[0,∞)v : \mathbb{R}^{3} \to[0,\infty) be bounded, measurable, radial, and supported in a ball of finite radius, with vv not zero almost everywhere. On the torus ΛL=(R/LZ)3\Lambda_L = (\mathbb{R}/L\mathbb{Z})^{3}, of volume V=L3V = L^{3}, let vL(x)=∑k∈Z3v(x+Lk)v_L(x) = \sum_{k\in\mathbb{Z}^{3}} v(x + Lk) and define

HN,L=−∑i=1NΔi+∑1≤i<j≤NvL(xi−xj)on Lsym2(ΛLN).H_{N,L} = -\sum_{i=1}^{N} \Delta_i + \sum_{1\leq i<j\leq N} v_L(x_i-x_j)\quad\text{on }L^2_{\mathrm{sym}}(\Lambda_L^N).

The units are ℏ2/(2mparticle)=kB=1\hbar^2/(2m_{\mathrm{particle}}) = k_B = 1. At T>0T > 0, the state is the canonical Gibbs state ΓN,L,T=e−HN,L/T/Tr⁡e−HN,L/T\Gamma_{N,L,T} = e^{-H_{N,L}/T}/\operatorname{Tr}e^{-H_{N,L}/T}; at T=0T = 0, it is the ground state. Write γN,L,T(1)\gamma^{(1)}_{N,L,T} for its one-particle density matrix, normalized to trace NN, and put u0=V−1/2u_0 = V^{-1/2}.

Theorem 1.1. For every potential vv as above there are constants ρ∗(v)>0\rho_*(v) > 0 and c∗(v)>0c_*(v) > 0 with the following property. For every 0<ρ<ρ∗(v)0 < \rho< \rho_*(v) there is L0(ρ,v)<∞L_0(\rho,v) < \infty such that, for every L≥L0(ρ,v)L \geq L_0(\rho,v), every integer N≥1N \geq1 satisfying ρ/2≤N/L3≤2ρ\rho/2 \leq N/L^3 \leq2\rho, and every 0≤T≤ρ20 \leq T \leq\rho^2,

⟨u0,γN,L,T(1)u0⟩N≥c∗(v).\frac{\langle u_0,\gamma^{(1)}_{N,L,T}u_0\rangle}{N} \geq c_*(v).

Consequently, for each such fixed density ρ\rho and fixed 0≤T≤ρ20 \leq T \leq\rho^2, every sequence with L→∞L \to\infty and N/L3→ρN/L^3 \to\rho has lower limiting condensate fraction at least c∗(v)c_*(v).

The volume threshold may depend on the density; the condensate lower bound does not. The Hamiltonian is the exact interacting Hamiltonian, and its potential is not rescaled with the number of particles. The conclusion is macroscopic occupation of the constant orbital with a positive lower bound throughout the admitted dilute interval. The zero-temperature state is unambiguous: positivity of the finite-volume heat kernel gives a unique bosonic ground state, as shown at the end of the proof.

Context and antecedents

The ideal-gas theory begins with Bose’s counting of light quanta [8] and Einstein’s extension to a monatomic ideal gas, including the condensation prediction in his second paper [15, 16]. Bogoliubov’s treatment of weakly interacting bosons introduced an approximate quasiparticle description based on macroscopic occupation of one mode [7].

For interacting particles, Penrose and Onsager formulated condensation through a macroscopic eigenvalue of the one-particle density matrix and applied this viewpoint to liquid helium [31]. Yang developed the broader framework of off-diagonal long-range order, covering Bose condensation and fermion pairing [36]. These criteria identify the order to be proved; establishing it for a specified interacting Hamiltonian remains a separate mathematical problem.

Rigorous lattice antecedents include Dyson, Lieb, and Simon’s low-temperature long-range order for the spin-12\frac{1}{2} nearest-neighbor quantum XY model on the simple cubic lattice in dimensions d≥3d \ge3 [14], and Kennedy, Lieb, and Shastry’s ground-state long-range order for all spins on hypercubic lattices in dimensions d≥2d \ge2 [26]. For spin-12\frac{1}{2}, the spin–hard-core-boson correspondence relates these results to condensation of half-filled lattice bosons. Passing to a continuum Hamiltonian with a fixed interaction and a prescribed density requires additional arguments.

The distinction between the thermodynamic and Gross–Pitaevskii limits is essential. Lieb and Seiringer proved complete condensation in the Gross–Pitaevskii limit, with the interaction scaled so that NaNa remains fixed, where aa is the scattering length [29]. Deuchert and Seiringer subsequently treated positive-temperature homogeneous gases with scattering length aN=avL/Na_N = a_vL/N, where ava_v is the scattering length of the unscaled potential, and controlled the one-particle density matrix of approximate Gibbs minimizers [11]. These results allow the interaction scale to vary with particle number. The problem considered here instead fixes the potential and a positive density before taking the volume to infinity.

The limits between Gross–Pitaevskii scaling and a fixed-density thermodynamic limit have several forms. Brennecke, Brooks, Caraci, and Oldenburg proved complete ground-state condensation in the Gross–Pitaevskii regime and beyond [9]. Fournais treated low-energy states on growing boxes in a joint dilute and increasing-volume limit [19], Theorem 1.2. Chong, Liang, and Nam gave simpler proofs of low-energy condensation using kinetic localization and Poincaré-type inequalities [10]. For the unit-box interaction N2−2κv(N1−κx)N^{2-2\kappa}v(N^{1-\kappa}x), rescaling to a fixed potential gives density N3κ−2N^{3\kappa-2}; the regimes κ<2/3\kappa< 2/3 therefore couple dilution to increasing particle number. Junge’s low-temperature canonical Gibbs-state result uses Neumann boxes whose size remains coupled to the dilute limit [25], Corollary 6.

The thermodynamic energy problem has a separate history. Dyson’s hard-sphere bounds and the leading dilute asymptotics of Lieb and Yngvason established the first-order energy scale [13, 30]. The next correction was predicted by Lee, Huang, and Yang’s pseudopotential calculation [27]. Fournais and Solovej proved the corresponding lower bound for nonnegative radial finite-range potentials, including hard cores [20], Theorems 1.1 and 1.3; recent upper bounds attain the same coefficient for hard spheres and for general nonnegative even finite-range potentials [3, 4]. These energy results, and low-temperature free-energy estimates for strong potentials [18], do not by themselves determine occupation of a single orbital: the one-particle kinetic gap tends to zero as the volume grows.

A distinct thermodynamic-limit result appears in Sütő’s two-step preprint [33]. Its Theorem 1.2 assumes nonnegativity both of the potential and of its Fourier transform, together with integrability, a Fourier-moment condition, and spatial decay, and states condensation above a temperature-dependent density threshold. Fourier positivity is an additional restriction: for example, a nonnegative spherical square barrier has a Fourier transform that changes sign. That result therefore does not cover all bounded nonnegative radial finite-range potentials, and its fixed-temperature threshold does not alone provide the joint low-density and low-temperature uniformity sought here.

Galanda and Pinamonti construct algebraic equilibrium states with a condensate background under quantitative convergence conditions for a spatially localized interaction [21], Theorem 6.8. Their subsequent analysis treats renormalized correlation functions in Gross–Pitaevskii scaling, with a zero-temperature limit in its final convergence theorem [22], Theorem 7.3. These constructions use a different state formulation and coupled interaction, regulator, and temperature limits from the fixed-potential canonical thermodynamic limit considered here.

The trajectory formulation descends from Feynman’s treatment of the Bose gas [17]; for the canonical Feynman–Kac representation and its symmetrization and one-particle normalizations, see [35]. The random-path comparison has a different ancestry. Benjamini, Pemantle, and Peres constructed paths with exponentially decaying intersection tails [5]. Häggström and Mossel developed a hierarchical random-drift construction with low predictability; its independent block variables are a close antecedent of the dyadic velocities used below [24]. Abbe, Massoulié, Montanari, Sly, and Srivastava used finite-endpoint path averages and overlap estimates for group synchronization [1]; Garban and Spencer used this approach for classical disordered-spin symmetry breaking along the Nishimori line [23]. Here the finite cell paths, their thickened intersection estimates, and the continuum bridge comparison require separate proofs.

How the comparison works

Let q0=⟨u0,γ(1)u0⟩/Nq_0 = \langle u_0, \gamma^{(1)}u_0\rangle/N. The Feynman–Kac formula expresses the partition function by positive weights on closed collections of paths. Replacing one matching endpoint by an independently integrated spatial point gives a positive measure μ\mu of total mass q0q_0. We construct a measure ν\nu by changing a short portion of closed paths, with mass at least a fixed a>0a > 0, and show that its density f=dν/dμf = \mathrm{d}\nu/\mathrm{d}\mu has bounded second moment. Cauchy–Schwarz then gives

a2≤q0∫f2 dμ.a^2 \le q_0 \int f^2 \,\mathrm{d}\mu.

Thus the main problem is a comparison of positive path measures.

Partition space into cells of side ss comparable to ρ−1/2\rho^{-1/2}, and change paths only during a time interval of length δ=s2\delta= s^2. The mean count m=Ns3/Vm = Ns^3/V is comparable to ρ−1/2\rho^{-1/2}, making many particle choices available in a typical cell as the density decreases, while the slab remains short compared with 1/T1/T throughout the positive-temperature range.

The local analysis must control simultaneous failures in specified families of cells. Energy and entropy estimates first give occupation tails and separation of most endpoints at the shorter scale r=ζρ−1/3r = \zeta\rho^{-1/3}, with ζ>0\zeta> 0 fixed and small. A particle is eligible when its endpoints are separated, its path stays near them during short initial and final time intervals, and it satisfies overall confinement and integrated interaction-score bounds for the path ensemble. The interacting bridges are not independent. A separate localized partition-function comparison bounds their joint trajectory failures, with a cost proportional to the volume of the tested cells. Together with the one-time estimates and score bounds, this makes specified sets of unusable cells unlikely.

Between two distant cells, choose a random lattice path, called a skeleton, whose encounters with an independent copy have bounded exponential moments. Here an encounter records a vertex within a fixed cell distance of the other path; a second estimate weights all vertices by exponentially decaying distance. These two geometric bounds are established independently of the gas in Section 8.1. Detour around unusable components. Select one eligible particle from each cell on the resulting simple path, and cyclically reassign their starting points. One end is opened and the selected bridges are sampled from their exactly normalized interacting law. This defines ν\nu.

The second moment involves two independently chosen paths in related configurations. Estimating both changes against the original closed configuration would incur a cost proportional to their lengths. Instead, a reverse insertion supplies a baseline in which contributions far from encounters cancel. Two effects remain small as ρ\rho decreases: an encounter of distinct separated bridges has interaction cost tending to zero at rate r−1/2r^{-1/2}, and coincident particle choices have probability of order 1/m1/m.

Changing trajectories also changes which cells are usable and which particles are eligible, so the two routes cannot be treated as independent of the gas. A stricter cell test in the reverse configuration controls these changes: away from encounters the selection weights agree, while rare components give a controlled list of possible detours. Keeping those selection weights throughout the comparison yields the required second-moment bound after averaging over the environment and the two paths.

Sections 3–7 prove the local analytic bounds. Section 8 constructs the paths and detours. Section 9 defines the change of measure, and Section 10 proves its second-moment estimate with all normalizations and selection constraints retained. Section 11 fixes the parameters in order and passes the uniform positive-temperature bound to zero temperature.

Scales and conventions

We use the Hamiltonian of Section 1 also on labelled coordinates, and suppress LL when it is fixed. We choose an everywhere nonnegative bounded Borel radial representative of vv vanishing outside its range ball. Changing this representative on a null set changes neither the operator nor the path integrals: at interior times the free relative positions have densities. Write RvR_v for a range bound, and use ∥v∥1,∥v∥∞\lVert v\rVert_1,\lVert v\rVert_\infty on R3\mathbb{R}^3. In formulas on the torus, vv abbreviates its periodization vLv_L; infinite-space norms always refer to the original potential.

The orthogonal symmetrizer is included exactly once in a trace kernel. If ktk_t is the labelled NN-particle kernel, then

ktsym(X,Y)=1N!∑π∈SNkt(X,πY),ZN=∫kβsym(X,X) dX.k_t^{\mathrm{sym}}(X,Y)=\frac{1}{N!}\sum_{\pi\in\mathfrak{S}_N} k_t(X,\pi Y),\qquad Z_N=\int k_\beta^{\mathrm{sym}}(X,X)\,\mathrm{d}X.

Thus integration over labelled coordinates carries no further factorial. We work with ρ/2≤N/V≤2ρ\rho/2\leq N/V\leq2\rho, 0<T≤ρ20<T\leq\rho^2, and β=T−1\beta=T^{-1}. Every volume restriction below is imposed at fixed ρ\rho, uniformly over this temperature interval. Constants C,c>0C,c>0 may change between occurrences and depend on vv and previously fixed cutoffs, but not on ρ,L,N,T\rho,L,N,T. The final order of those cutoff choices is recorded in Section 11.

We use a periodic grid G=(Z/nZ)3\mathcal{G}=(\mathbb{Z}/n\mathbb{Z})^3 of equal cubes (fix the assignment at faces), with

n=⌊LKρ−1/2⌋,s=L/n∈[Kρ−1/2,2Kρ−1/2],M=n3,m=N/M.n=\left\lfloor\frac{L}{K\rho^{-1/2}}\right\rfloor,\qquad s=L/n\in[K\rho^{-1/2},2K\rho^{-1/2}],\qquad M=n^3,\qquad m=N/M.

Here K≥1K\geq1 is a fixed large constant chosen below. Thus ρs3/2≤m≤2ρs3\rho s^3/2\leq m\leq2\rho s^3.

A union UU of u≥1u\geq1 cells has volume ∣U∣=us3|U|=us^3. A neighborhood out to distance hshs, h≥0h\geq0, can be covered by at most C(h+2)3uC(h+2)^3u cells, including on the torus. Physical distances d(⋅,⋅)d(\cdot,\cdot) are Euclidean torus distances unless indicated otherwise. Cell index distances will use the periodic sup norm. For a function pp of position put np(X)=∑ip(xi)n_p(X)=\sum_i p(x_i) on configurations (also the multiplication operator); similarly nUn_U for counting particles in UU.

Energy and free-energy estimates

This section gives the particle-number costs needed to localize the gas. Throughout, 0<T≤ρ20<T\leq\rho^2, β=T−1\beta=T^{-1}, and ρ/2≤N/V≤2ρ\rho/2\leq N/V\leq2\rho. All statements hold after decreasing a potential-dependent upper bound on ρ\rho and increasing the volume threshold at each fixed density. The Hamiltonian with a bounded external potential −W-W is denoted by Hj,L(−W)H_{j,L}^{(-W)}; its symmetric partition function and free energy are Zj(−W)Z_j^{(-W)} and Fj(−W)=−Tlog⁡Zj(−W)F_j^{(-W)}=-T\log Z_j^{(-W)}. We set Z0=1Z_0=1 and F0=0F_0=0. For a trace-one state σ\sigma, write F(−W)(σ)=Tr⁡H(−W)σ−TS(σ)\mathcal{F}^{(-W)}(\sigma)=\operatorname{Tr} H^{(-W)}\sigma-T S(\sigma). Here S(σ)=−Tr⁡(σlog⁡σ)S(\sigma)=-\operatorname{Tr}(\sigma\log\sigma) is the von Neumann entropy, with 0log⁡0=00\log0=0. Constants may depend on vv, and later on already fixed dimensionless parameters, but never on ρ\rho, LL, NN, TT.

Lemma 3.1 (A Neumann cell bound). There are b0,cv>0b_0,c_v>0, depending only on the fixed potential, such that for a cube QQ of side b≥b0b\ge b_0, every y∈Qy\in Q, and every f∈H1(Q)f\in H^1(Q),

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