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WorksPhysics and Astronomy

Nearly Isotropic Vortex Solid in (La,Pr)3Ni2O7\mathbf{(La,Pr)_{3}Ni_{2}O_{7}} Thin Films

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Abstract · v1

The discovery of superconductivity in bulk bilayer nickelates has established a new platform for exploring high-TcT_c superconductivity beyond the cuprates. The role of the Ni 3dz23d_{z^2}-derived γγ band in the superconductivity of bilayer nickelates remains unresolved. By performing simultaneous resistance and diamagnetism measurements on (La,Pr)3_3Ni2_2O7_7 thin films, we map the vortex melting phase diagram for both in-plane and out-of-plane magnetic fields. For H∥cH\parallel c, the geometric confinement effect gives rise to pancake vortices. Remarkably, the anisotropy parameter of the vortex melting field γHm≡Hmab/Hmcγ_{H_m} \equiv H_m^{ab}/H_m^c decreases monotonically with decreasing temperature and approaches unity at low temperatures. Within the anisotropic Ginzburg–Landau scaling, Hmab/Hmc=ρsab/ρscH_m^{ab}/H_m^c = \sqrt{ρ_s^{ab}/ρ_s^c} tracks the superfluid-density anisotropy. Such a vortex solid implies a nearly isotropic superfluid density, which is irreconcilable with the strictly two-dimensional 3dx2−y23d_{x^2-y^2}-derived bands, but naturally explained by a substantial interlayer superfluid contribution from the 3dz23d_{z^2}-derived γγ band. Our results provide thermodynamic evidence for a substantial contribution of the γγ band to superconductivity in bilayer nickelate thin films.

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